Manipulating charge transfer excited state relaxation and spin crossover in iron coordination complexes with ligand substitution† †Electronic supplementary information (ESI) available. See DOI: 10.1039/c6sc03070j Click here for additional data file.

نویسندگان

  • Wenkai Zhang
  • Kasper S. Kjær
  • Roberto Alonso-Mori
  • Uwe Bergmann
  • Matthieu Chollet
  • Lisa A. Fredin
  • Ryan G. Hadt
  • Robert W. Hartsock
  • Tobias Harlang
  • Thomas Kroll
  • Katharina Kubiček
  • Henrik T. Lemke
  • Huiyang W. Liang
  • Yizhu Liu
  • Martin M. Nielsen
  • Petter Persson
  • Joseph S. Robinson
  • Edward I. Solomon
  • Zheng Sun
  • Dimosthenis Sokaras
  • Tim B. van Driel
  • Tsu-Chien Weng
  • Diling Zhu
  • Kenneth Wärnmark
  • Villy Sundström
  • Kelly J. Gaffney
چکیده

PULSE Institute, SLAC National Accelerato Park, California 94025, USA. E-mail: kaspe edu Department of Chemical Physics, Lund Univ Centre for Molecular Movies, Department of DK-2800, Lyngby, Denmark LCLS, SLAC National Accelerator Laborato Theoretical Chemistry Division, Lund Unive Department of Chemistry, Stanford Univers Max Planck Institute for Biophysical Chem SSRL, SLAC National Accelerator Laborator Centre for Analysis and Synthesis, Departme 124, 22100 Lund, Sweden † Electronic supplementary informa 10.1039/c6sc03070j ‡ These authors have contributed equally Cite this: Chem. Sci., 2017, 8, 515

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Manipulating charge transfer excited state relaxation and spin crossover in iron coordination complexes with ligand substitution.

Developing light-harvesting and photocatalytic molecules made with iron could provide a cost effective, scalable, and environmentally benign path for solar energy conversion. To date these developments have been limited by the sub-picosecond metal-to-ligand charge transfer (MLCT) electronic excited state lifetime of iron based complexes due to spin crossover - the extremely fast intersystem cro...

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عنوان ژورنال:

دوره 8  شماره 

صفحات  -

تاریخ انتشار 2017